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Preparation of polymers and copolymers having predictable molecular
weights and well-defined architectures can be accomplished via atom transfer
radical polymerization (ATRP). However, the high concentration of transition
metal catalysts required for the successful reaction causes those same
catalysts to precipitate with the product, often leading to highly
problematic levels of contamination. Thus, the technical challenge faced in
the polymer community is how to reduce the quantity of residual catalyst in
the product. Methods currently in use include post-purification washing,
reprecipitation, and absorption. These methodologies lead to higher cost and
loss of polymer as well as the ever present difficulty with regard to
scaling up the reaction from the bench/laboratory setting to full-scale
industrial use.
Researchers in the University of Wyoming have developed and filed a patent
application on a novel method to increase catalyst activity allowing for
decreased catalyst concentration. Ultimately this catalyst has enhanced
activity and smaller concentrations which allow it to remain in the product
with very small economic impact and negligible impact on product quality.
Tests have shown that this new catalyst has very high activity for methyl
acrylate (MA), methyl methacrylate (MMA), and styrene (St) polymerizations.
At 1 mol % catalyst (relative to initiator) is sufficient to produce these
products, all having well-controlled molecular weights and low
polydispersities (1.15, 1.24, and 1.18 for MA, MMA, and St respectively).
The level of catalyst concentration approximately 30 ppm followed by one
precipation which reduced the level of catalyst contamination to merely
several ppm. These extremely low levels require no post-purification or
catalyst recycling in an industrial setting. Thus, this new catalyst, has
very promising results for industrial ATRP polymer/copolymer reactions.
CONTACT INFORMATION
If your company would like to learn more about this technology and how your
company may help us develop it or apply it in commercial situations, please
contact the director of the University of Wyoming Research Products Center,
Davona Douglass.
Research Products Center
Dept. 3672
1000 E. University Ave.
Laramie, WY 82071
(307)766-2520
Fax: (307) 766-2530
e-mail: WyomingInvents@uwyo.edu